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A novel tracer technique to quantify the atmospheric flux of trace elements to remote ocean regions ArchiMer
Kadko, David; Landing, William M.; Shelley, Rachel.
Atmospheric input into the global ocean constitutes an important budgetary component of numerous chemical species and plays a key role in controlling biogeochemical processes in the ocean. Assessment of this input is difficult, however, because measurements of deposition rates to the ocean, particularly in remote areas, are rare and susceptible to problems of temporal and spatial variability. While the collection and analysis of aerosol samples is somewhat routine, the chemical concentration data collected from ship board or land-based aerosol samplers in and of themselves cannot yield the deposition flux of trace elements; a method is required to transform concentration measurements into flux. The ability to derive the atmospheric flux of Be-7 from its...
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Ano: 2015 URL: https://archimer.ifremer.fr/doc/00266/37727/35737.pdf
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Inputs and processes affecting the distribution of particulate iron in the North Atlantic along the GEOVIDE (GEOTRACES GA01) section ArchiMer
Gourain, Arthur; Planquette, Helene; Cheize, Marie; Lemaitre, Nolwenn; Menzel Barraqueta, Jan-lukas; Shelley, Rachel; Lherminier, Pascale; Sarthou, Geraldine.
The GEOVIDE cruise (May–June 2014, R/V Pourquoi Pas?) aimed to provide a better understanding on trace metal biogeochemical cycles in the North Atlantic. As particles play a key role in the global biogeochemical cycle of trace elements in the ocean, we discuss the distribution of particulate iron (PFe), in light of particulate aluminium (PAl), manganese (PMn) and phosphorus (PP) distributions. Overall, 32 full vertical profiles were collected for trace metal analyses, representing more than 500 samples. This resolution provides a solid basis for assessing concentration distributions, elemental ratios, size-fractionation, or adsorptive scavenging processes in key areas of the thermohaline circulation. Total particulate iron (PFe) concentrations ranged from...
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Ano: 2019 URL: https://archimer.ifremer.fr/doc/00485/59676/62747.pdf
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Regional trends in the fractional solubility of Fe and other metals from North Atlantic aerosols (GEOTRACES cruises GA01 and GA03) following a two-stage leach ArchiMer
Shelley, Rachel; Landing, William M.; Ussher, Simon J.; Planquette, Helene; Sarthou, Geraldine.
The fractional solubility of aerosol-derived trace elements deposited to the ocean surface is a key parameter of many marine biogeochemical models. Despite this, it is currently poorly constrained, in part due to the complex interplay between the various processes that govern the solubilisation of aerosol trace elements. In this study, we used a sequential two-stage leach to investigate the regional variability in fractional solubility of a suite of aerosol trace elements (Al, Ti, Fe, Mn, Co, Ni, Cu, Zn, Cd, and Pb) from samples collected during three GEOTRACES cruises to the North Atlantic Ocean (GA01, GA03-2010, and GA03-2011). We present aerosol trace element solubility data from two sequential leaches that provide a solubility window, covering a...
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Ano: 2018 URL: https://archimer.ifremer.fr/doc/00439/55041/56473.pdf
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Dissolved iron in the North Atlantic Ocean and Labrador Sea along the GEOVIDE section (GEOTRACES section GA01) ArchiMer
Tonnard, Manon; Planquette, Hélène; Bowie, Andrew R.; Van Der Merwe, Pier; Gallinari, Morgane; Desprez De Gésincourt, Floriane; Germain, Yoan; Gourain, Arthur; Benetti, Marion; Reverdin, Gilles; Tréguer, Paul; Boutorh, Julia; Cheize, Marie; Menzel Barraqueta, Jan-lukas; Pereira-contreira, Leonardo; Shelley, Rachel; Lherminier, Pascale; Sarthou, Géraldine.
Dissolved Fe (DFe) samples from the GEOVIDE voyage (GEOTRACES GA01, May–June 2014) in the North Atlantic Ocean were analysed using a SeaFAST-picoTM coupled to an Element XR HR-ICP-MS and provided interesting insights on the Fe sources in this area. Overall, DFe concentrations ranged from 0.09 ± 0.01 nmol L−1 to 7.8 ± 0.5 nmol L−1. Elevated DFe concentrations were observed above the Iberian, Greenland and Newfoundland Margins likely due to riverine inputs from the Tagus River, meteoric water inputs and sedimentary inputs. Air-sea interactions were suspected to be responsible for the increase in DFe concentrations within subsurface waters of the Irminger Sea due to deep convection occurring the previous winter, that provided iron-to-nitrate ratios sufficient...
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Ano: 2020 URL: https://archimer.ifremer.fr/doc/00441/55233/56714.pdf
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Dissolved Pb and Pb isotopes in the North Atlantic from the GEOVIDE transect (GEOTRACES GA-01) and their decadal evolution ArchiMer
Zurbrick, Cheryl M.; Boyle, Edward A.; Kayser, Richard J.; Reuer, Matthew K.; Wu, Jinfeng; Planquette, Helene; Shelley, Rachel; Boutorh, Julia; Cheize, Marie; Contreira, Leonardo; Barraqueta, Jan-lukas Menzel; Lacan, Francois; Sarthou, Geraldine.
During the 2014 GEOVIDE transect, seawater samples were collected for dissolved Pb and Pb isotope analysis. These samples provide a high-resolution "snapshot" of the source regions for the present Pb distribution in the North Atlantic Ocean. Some of these stations were previously occupied for Pb from as early as 1981, and we compare the 2014 data with these older data, some of which are reported here for the first time. Lead concentrations were highest in subsurface Mediterranean Water (MW) near the coast of Portugal, which agrees well with other recent observations by the US GEOTRACES program (Noble et al., 2015). The recently formed Labrador Sea Water (LSW) between Greenland and Nova Scotia is much lower in Pb concentration than the older LSW found in...
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Ano: 2018 URL: https://archimer.ifremer.fr/doc/00456/56760/58607.pdf
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Mercury distribution and transport in the North Atlantic Ocean along the GEOTRACES-GA01 transect ArchiMer
Cossa, Daniel; Heimburger, Lars-eric; Perez, Fiz F; Garcia-ibanez, Maria Isabel; Sonke, Jeroen E.; Planquette, Helene; Lherminier, Pascale; Boutorh, Julia; Cheize, Marie; Barraqueta, Jan Lukas Menzel; Shelley, Rachel; Sarthou, Geraldine.
We report here the results of total mercury (HgT) determinations along the 2014 GEOTRACES GEOVIDE cruise (GA01 transect) in the North Atlantic Ocean (NA) from Lisbon (Portugal) to the Labrador coast (Canada). Ninety-seven percent of the HgT concentrations of unfiltered samples (HgTUNF) ranged between 0.16 and 1.00 pmol L−1. The geometric mean was 0.51 pmol L−1 for the 535 samples analysed. The dissolved fraction (< 0.45 μm) of HgT, determined on 141 samples, averaged 78 % of the HgTUNF for the whole water column. HgTUNF concentrations increased eastwards and with depth from Greenland to Europe and from sub-surface to bottom waters, respectively. The Hg distribution mirrored that of dissolved oxygen concentration, with highest HgTUNF levels associated...
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Ano: 2018 URL: https://archimer.ifremer.fr/doc/00412/52303/53071.pdf
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The GEOTRACES Intermediate Data Product 2017 ArchiMer
Schlitzer, Reiner; Anderson, Robert F.; Dodas, Elena Masferrer; Lohan, Maeve; Geibere, Walter; Tagliabue, Alessandro; Bowie, Andrew; Jeandel, Catherine; Maldonado, Maria T.; Landing, William M.; Cockwell, Donna; Abadie, Cyril; Abouchami, Wafa; Achterberg, Eric P.; Agather, Alison; Aguliar-islas, Ana; Van Aken, Hendrik M.; Andersen, Morten; Archer, Corey; Auro, Maureen; De Baar, Hein J.; Baars, Oliver; Baker, Alex R.; Bakker, Karel; Basak, Chandranath; Baskaran, Mark; Bates, Nicholas R.; Bauch, Dorothea; Van Beek, Pieter; Behrens, Melanie K.; Black, Erin; Bluhm, Katrin; Bopp, Laurent; Bouman, Heather; Bowman, Katlin; Bown, Johann; Boyd, Philip; Boye, Marie; Boyle, Edward A.; Branellec, Pierre; Bridgestock, Luke; Brissebrat, Guillaume; Browning, Thomas; Bruland, Kenneth W.; Brumsack, Hans-juergen; Brzezinski, Mark; Buck, Clifton S.; Buck, Kristen N.; Buesseler, Ken; Bull, Abby; Butler, Edward; Cai, Pinghe; Camara Mor, Patricia; Cardinal, Damien; Carlson, Craig; Carrasco, Gonzalo; Casacuberta, Nuria; Casciotti, Karen L.; Castrillejo, Maxi; Chamizo, Elena; Chance, Rosie; Charette, Matthew A.; Chaves, Joaquin E.; Cheng, Hai; Chever, Fanny; Christl, Marcus; Church, Thomas M.; Closset, Ivia; Colman, Albert; Conway, Tim M.; Cossa, Daniel; Croot, Peter; Cullen, Jay T.; Cutter, Gregory A.; Daniels, Chris; Dehairs, Frank; Deng, Feifei; Dieu, Huong Thi; Duggan, Brian; Dulaquais, Gabriel; Dumousseaud, Cynthia; Echegoyen-sanz, Yolanda; Edwards, R. Lawrence; Ellwood, Michael; Fahrbach, Eberhard; Fitzsimmons, Jessica N.; Flegal, A. Russell; Fleisher, Martin Q.; Van De Flierdt, Tina; Frank, Martin; Friedrich, Jana; Fripiat, Francois; Froellje, Henning; Galer, Stephen J. G.; Gamo, Toshitaka; Ganeshram, Raja S.; Garcia-orellana, Jordi; Garcia-solsona, Ester; Gault-ringold, Melanie; George, Ejin; Gerringa, Loes J. A.; Gilbert, Melissa; Godoy, Jose M.; Goldstein, Steven L.; Gonzalez, Santiago R.; Grissom, Karen; Hammerschmidt, Chad; Hartman, Alison; Hassler, Christel S.; Hathorne, Ed C.; Hatta, Mariko; Hawco, Nicholas; Hayes, Christopher T.; Heimburger, Lars-eric; Helgoe, Josh; Heller, Maija Iris; Henderson, Gideon M.; Henderson, Paul B.; Van Heuven, Steven; Ho, Peng; Horner, Tristan J.; Hsieh, Yu-te; Huang, Kuo-fang; Humphreys, Matthew P.; Isshiki, Kenji; Jacquot, Jeremy E.; Janssen, David J.; Jenkins, William J.; John, Seth; Jones, Elizabeth M.; Jones, Janice L.; Kadko, David C.; Kayser, Rick; Kenna, Timothy C.; Khondoker, Roulin; Kim, Taejin; Kipp, Lauren; Klar, Jessica K.; Klunder, Maarten; Kretschmer, Sven; Kumamoto, Yuichiro; Laan, Patrick; Labatut, Marie; Lacan, Francois; Lam, Phoebe J.; Lambelet, Myriam; Lamborg, Carl H.; Le Moigne, Frederic A. C.; Le Roy, Emilie; Lechtenfeld, Oliver J.; Lee, Jong-mi; Lherminier, Pascale; Little, Susan; Lopez-lora, Mercedes; Lu, Yanbin; Masque, Pere; Mawji, Edward; Mcclain, Charles R.; Measures, Christopher; Mehic, Sanjin; Barraqueta, Jan-lukas Menzel; Van Der Merwe, Pier; Middag, Rob; Mieruch, Sebastian; Milne, Angela; Minami, Tomoharu; Moffett, James W.; Moncoiffe, Gwenaelle; Moore, Willard S.; Morris, Paul J.; Morton, Peter L.; Nakaguchi, Yuzuru; Nakayama, Noriko; Niedermiller, John; Nishioka, Jun; Nishiuchi, Akira; Noble, Abigail; Obata, Hajime; Ober, Sven; Ohnemus, Daniel C.; Van Ooijen, Jan; O'Sullivan, Jeanette; Owens, Stephanie; Pahnke, Katharina; Paul, Maxence; Pavia, Frank; Pena, Leopoldo D.; Petersh, Brian; Planchon, Frederic; Planquette, Helene; Pradoux, Catherine; Puigcorbe, Viena; Quay, Paul; Queroue, Fabien; Radic, Amandine; Rauschenberg, S.; Rehkamper, Mark; Rember, Robert; Remenyi, Tomas; Resing, Joseph A.; Rickli, Joerg; Rigaud, Sylvain; Rijkenberg, Micha J. A.; Rintoul, Stephen; Robinson, Laura F.; Roca-marti, Montserrat; Rodellas, Valenti; Roeske, Tobias; Rolison, John M.; Rosenberg, Mark; Roshan, Saeed; Van Der Loaff, Michiel M. Rutgers; Ryabenko, Evgenia; Saito, Mak A.; Salt, Lesley A.; Sanial, Virginie; Sarthou, Geraldine; Schallenberg, Christina; Schauer, Ursula; Scher, Howie; Schlosser, Christian; Schnetger, Bernhard; Scott, Peter; Sedwick, Peter N.; Semiletov, Igor; Shelley, Rachel; Sherrell, Robert M.; Shiller, Alan M.; Sigman, Daniel M.; Singh, Sunil Kumar; Slagter, Hans A.; Slater, Emma; Smethie, William M.; Snaith, Helen; Sohrin, Yoshiki; Sohst, Bettina; Sonke, Jeroen E.; Speich, Sabrina; Steinfeldt, Reiner; Stewart, Gillian; Stichel, Torben; Stirling, Claudine H.; Stutsman, Johnny; Swarr, Gretchen J.; Swift, James H.; Thomas, Alexander; Thorne, Kay; Till, Claire P.; Till, Ralph; Townsend, Ashley T.; Townsend, Emily; Tuerena, Robyn; Twining, Benjamin S.; Vance, Derek; Velazquez, Sue; Venchiarutti, Celia; Villa-alfageme, Maria; Vivancos, Sebastian M.; Voelker, Antje H. L.; Wake, Bronwyn; Warner, Mark J.; Watson, Ros; Van Weerlee, Evaline; Weigand, M. Alexandra; Weinstein, Yishai; Weiss, Dominik; Wisotzki, Andreas; Woodward, E. Malcolm S.; Wu, Jingfeng; Wu, Yingzhe; Wuttig, Kathrin; Wyatt, Neil; Xiang, Yang; Xie, Ruifang C.; Xue, Zichen; Yoshikawa, Hisayuki; Zhang, Jing; Zhang, Pu; Zhao, Ye; Zheng, Linjie; Zheng, Xin-yuan; Zieringer, Moritz; Zimmer, Louise A.; Ziveri, Patrizia; Zunino, Patricia; Zurbrick, Cheryl.
The new IDP2017 is a significant improvement over the earlier IDP2014 and roughly doubles the number of included cruises, stations, samples and parameters. The IDP2017 is a truly international product containing data from 326 researchers from 25 countries. The IDP2017 provides data for the Pacific Ocean, and the Mediterranean and Black seas, in addition to Atlantic, Arctic and Indian Oceans that were already represented in the previous data product. For the first time, the IDP2017 contains significant amounts of biogeochemistry data as well as TEI data for aerosols and rain. As before, users can obtain complete IDP2017 data sets as bulk downloads. Alternatively, there is now a customisable online data extraction service that allows data selections by...
Tipo: Text Palavras-chave: GEOTRACES; Trace elements; Isotopes; Electronic atlas; IDP2017.
Ano: 2018 URL: https://archimer.ifremer.fr/doc/00442/55362/56877.pdf
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Aluminium in the North Atlantic Ocean and the Labrador Sea (GEOTRACES GA01 section): roles of continental inputs and biogenic particle removal ArchiMer
Barraqueta, Jan-lukas Menzel; Schlosser, Christian; Planquette, Helene; Gourain, Arthur; Cheize, Marie; Boutorh, Julia; Shelley, Rachel; Pereira, Leonardo Contreira; Gledhill, Martha; Hopwood, Mark J.; Lacan, Francois; Lherminier, Pascale; Sarthou, Geraldine; Achterberg, Eric P..
The distribution of dissolved aluminium (dAl) in the water column of the North Atlantic and Labrador Sea was studied along GEOTRACES section GA01 to unravel the sources and sinks of this element. Surface water dAl concentrations were low (median of 2.5 nM) due to low aerosol deposition and removal by phytoplankton. However, surface water dAl concentrations were enhanced on the Iberian and Greenland shelves (up to 30.9 nM) due to continental inputs (rivers, glacial flour and ice melt). A negative correlation was observed between dAl in surface waters and primary production, phytoplankton community structure and biogenic opal production. The abundance of diatoms exerted a significant (p < 0.01) control on the surface particulate Al (pAl) to dAl ratios by...
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Ano: 2018 URL: https://archimer.ifremer.fr/doc/00422/53359/54197.pdf
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Atmospheric deposition fluxes over the Atlantic Ocean: a GEOTRACES case study ArchiMer
Menzel Barraqueta, Jan-lukas; Klar, Jessica K.; Gledhill, Martha; Schlosser, Christian; Shelley, Rachel; Planquette, Helene; Wenzel, Bernhard; Sarthou, Geraldine; Achterberg, Eric P..
Atmospheric deposition is an important source of micronutrients to the ocean, but atmospheric deposition fluxes remain poorly constrained in most ocean regions due to the limited number of field observations of wet and dry atmospheric inputs. Here we present the distribution of dissolved aluminium (dAl), as a tracer of atmospheric inputs, in surface waters of the Atlantic Ocean along GEOTRACES sections GA01, GA06, GA08, and GA10. We used the surface mixed-layer concentrations of dAl to calculate atmospheric deposition fluxes using a simple steady state model. We have optimized the Al fractional aerosol solubility, the dAl residence time within the surface mixed layer and the depth of the surface mixed layer for each separate cruise to calculate the...
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Ano: 2019 URL: https://archimer.ifremer.fr/doc/00491/60227/63598.pdf
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Atmospheric aerosoldeposition fluxes over the Atlantic Ocean: A GEOTRACES case study ArchiMer
Menzel Barraqueta, Jan-lukas; Klar, Jessica K.; Gledhill, Martha; Schlosser, Christian; Shelley, Rachel; Planquette, Helene; Wenzel, Bernhard; Sarthou, Geraldine; Achterberg, Eric P..
Atmospheric deposition is an important source of micronutrients to the ocean, but atmospheric deposition fluxes remain poorly constrained in most ocean regions due to the limited number of field observations of wet and dry atmospheric inputs. Here we present the distribution of dissolved aluminium (dAl), as a tracer of atmospheric inputs, in surface waters of the Atlantic Ocean along GEOTRACES sections GA01, GA06, GA08, and GA10. We used the surface mixed layer concentrations of dAl to calculate atmospheric deposition fluxes using a simple steady state model. We have optimized the aerosol Al fractional solubility, dAl residence time within the surface mixed layer and depth of the surface mixed layer for each separate cruise to calculate the atmospheric...
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Ano: 2019 URL: https://archimer.ifremer.fr/doc/00485/59675/62745.pdf
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